$\begin{aligned}
& \overrightarrow{\mathrm{c}}=3 \overrightarrow{\mathrm{a}}+6 \overrightarrow{\mathrm{b}}+9(\overrightarrow{\mathrm{a}} \times \overrightarrow{\mathrm{b}}) \
& \sin ^{-1}\left(\frac{\sqrt{65}}{9}\right) \Rightarrow \sin \theta=\frac{\sqrt{65}}{9} \Rightarrow \cos \theta=\frac{4}{9} \
& \overrightarrow{\mathrm{c}} \cdot \overrightarrow{\mathrm{a}}=3|\overrightarrow{\mathrm{a}}|^2+6 \vec{a} \cdot \vec{b}=3+\frac{6 \cdot 4}{9}=\frac{51}{9} \
& \overrightarrow{\mathrm{c}} \cdot \vec{a}=3 \overrightarrow{\mathrm{a}} \cdot \overrightarrow{\mathrm{b}}+6|\overrightarrow{\mathrm{~b}}|^2=\frac{3 \cdot 4}{9}+6=\frac{22}{3} \
& \therefore 9(\overrightarrow{\mathrm{c}} \cdot \overrightarrow{\mathrm{a}})-3(\overrightarrow{\mathrm{c}} \cdot \vec{b})=51-22=29
\end{aligned}$